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논문 기본 정보

자료유형
학술저널
저자정보
김민석 (한국과학기술원) 한솔찬 (Physical and Life Sciences Directorate, Lawrence Livermore National Laboratory) 윤종일 (한국과학기술원)
저널정보
한국원자력학회 Nuclear Engineering and Technology Nuclear Engineering and Technology Vol.56 No.9
발행연도
2024.9
수록면
3,942 - 3,949 (8page)
DOI
10.1016/j.net.2024.04.041

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This study focuses on investigating the chemical degradation characteristics of cementitious barriers used in lowand intermediate-level radioactive waste repository by reactive transport modeling. The impact of the blending with supplementary cementitious materials (SCMs) in the barriers on the chemical degradation was evaluated to find the optimum barrier design. A number of different barrier designs were examined by replacing ordinary Portland cement (OPC) by SCMs (i.e., fly ash, silica fume, and blast-furnace slag). The simulation results showed that silica fume blended barrier has better durability against chemical degradation by rainwater compared to fly ash or blast-furnace slag blended barriers. In addition, the chemical durability of silica fume-based barrier increased with increasing replacement level up to about 20 %. It seems that the amount of formed calcium silicate hydrate (CSH) in the initial cement-based barrier highly affects the overall chemical durability. The newly developed reactive transport model demonstrated its capability for understanding the barrier performance and investigating the optimal design of the barrier system.

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