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논문 기본 정보

자료유형
학술저널
저자정보
Min Sung Kim (Korea Basic Science Institute) Lei Zhou (University of Chinese Academy of Sciences) Mira Choi (Korea Basic Science Institute) Yunlin Zhang (University of Chinese Academy of Sciences) Yongqiang Zhou (University of Chinese Academy of Sciences) Kyoung-Soon Jang (Korea Basic Science Institute)
저널정보
한국질량분석학회 Mass Spectrometry Letters Mass Spectrometry Letters Vol.12 No.4
발행연도
2021.12
수록면
192 - 199 (8page)

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초록· 키워드

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Alpine glaciers harbor a large quantity of bio-labile dissolved organic matter (DOM), which plays a pivotal role in global carbon cycling as glacial-fed streams are headwaters of numerous large rivers. To understand the complexity, origin, and fate of DOM in glaciers and downstream-linked streams and lakes, we elucidated the molecular composition of DOM in two different Tibetan Plateau glaciers, eight glacial-fed streams and five lakes, using an ultrahigh-resolution 15 Tesla Fourier transform ion cyclotron resonance (FT-ICR) mass spectrometer. The compositional changes of the DOM samples revealed that glacier DOM mostly exhibited sulfur-containing organic compounds (CHOS species). We also found that aliphatic formulae contributed more than 50% of the total abundance of assigned molecules in glacier samples, and those compounds were significantly related to CHOS species. The CHO proportions of glacial-fed streams and lakes samples increased with increasing distance from glacial terminals. The relative contribution of terrestrial-derived organics (i.e., lignins and tannins) declined while microbialoriginated organics (aliphatics) increased with increasing elevation. This suggested the gradual input of allochthonous materials from non-glacial environment and the degradation of microbe-derived compounds along lower elevations. Alpine glaciers are retreating as a result of climate change and they nourished numerous streams, rivers, and downstream-linked lakes. Therefore, the interpretations of the detailed molecular changes in glacier ice, glacial-fed streams, and alpine lakes on the Tibetan Plateau could provide broad insights for understanding the biogeochemical cycling of glacial DOM and assessing how the nature of DOM impacts fluvial ecosystems.

목차

Abstract
Introduction
Materials and Methods
Results and Discussion
Conclusions
References

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