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논문 기본 정보
- 자료유형
- 학술저널
- 저자정보
- 발행연도
- 2019.1
- 수록면
- 105 - 116 (12page)
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Three-dimensional (3D) graphene-based materials have attracted much attention in the field of supercapacitors for their large surface areas and fast electronic conductivity capability. Faradaic pseudo-capacitance materials inside the architecture can enlarge the electrochemical performance of the electrode. Additionally, metal porphyrins are negative electrode active materials for supercapacitors as they have potential high pseudo-capacitance, conductivity and N-doping. The design and preparation of the 3D cobalt-porphyrin modified graphene hydrogels (3D CoP/GHs) is an interesting topic. Here, we have fabricated the 3D CoP/GH by a two-step method. The composite electrode reaches a specific capacitance of 335 F g -1, twice that of pure GHs. At the same time, resistance of the electrode material decreases and the ion transfer is accelerated due to the addition of cobalt-porphyrin. After 10 000 cycles, the 3D CoP/GH maintains its stable specific capacitance retention of 94.11% indicating its excellent cycle life. The cycle life is much better than that of a hydrogel that has not been doped (81.63%) according to our previous work. Then we fabricated an asymmetrical supercapacitor which uses both the 3D CoP/GH and GH as the two electrodes (3D CoP/GHjjGH), and reaches an outstanding energy density of 30.40 Wh kg -1 at a current density of 1 A g -1 while the power density is 749.5 W kg -1.
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